The two players meet again when their countries go head-to-head in the semi-final of the Nations League, just five days after Liverpool beat Tottenham 2-0 in the Champions League final.
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Kane was underwhelming on his return from injury in Madrid, failing to escape the close attention of Van Dijk, who was imperious once again.
And Cascarino, writing in his column for the Times, says Van Dijk would be delighted if Kane starts again in Portugal.